109 – NASA Decision Support: Monitoring Air Quality Effects of Anthropogenic Emissions Reductions and Estimating Emissions from Natural Sources
Principal Investigator(s): D. Allen
An accurate specification of anthropogenic and natural emissions is crucial for determining the impact of emission perturbations on air quality. However, when this project began, lightning-NO emissions, a substantial contributor to tropospheric NO2 columns over the United States during the summertime, were not included in the Community Multiscale Air Quality (CMAQ) model used by the Environmental Protection Agency. The first goal of this project was to add lightning-NO emissions to CMAQ. Simulations with lightning-NO emissions provide more accurate estimates of nitrogen deposition and are useful for top down estimates of anthropogenic emissions. The second goal of this project was to use tropospheric nitrogen dioxide (NO2) columns retrieved from the Ozone Monitoring Instrument (OMI) aboard NASA’s Aura satellite to refine emissions of nitric oxide (NO) by microbial activity in soils calculated by the Biogenic Emission Inventory System (BEIS) that is used within the EPA’s Community Multiscale Air Quality Model (CMAQ).
Lightning-NO emissions in the CMAQ model were parameterized using a previously developed method that utilizes the relationship between flash rate and convective precipitation rate. The resulting flash rate distributions were scaled so that monthly average model flash rates match observed monthly average flash rates where the “observed” flash rates were determined using National Lightning Detection Network (NLDN) cloud-to-ground (CG) flash rates for the months of interest and climatological IC (intracloud)/CG ratios. CMAQ simulations were run with the improved source distributions for lightning-NO. Results were evaluated and the resulting algorithm is included as an option in the most recent release of CMAQ.
In order to evaluate how well CMAQ captures changes in NO2 columns associated with soil-NO emissions from BEIS, we compared changes in modeled and OMI-retrieved columns following precipitation events. Our goal was to determine if changes in NO2 columns associated with soil-NO emissions were visible in the OMI data set and if the observed changes were consistent with what was modeled via simulations with CMAQ. In order to put bounds on the emissions, we also performed CMAQ simulations with no soil-NO emissions and with doubled soil-NO emissions.